Articles | Volume 9, issue 2
https://doi.org/10.5194/soil-9-399-2023
https://doi.org/10.5194/soil-9-399-2023
Original research article
 | 
11 Jul 2023
Original research article |  | 11 Jul 2023

Validating plutonium-239+240 as a novel soil redistribution tracer – a comparison to measured sediment yield

Katrin Meusburger, Paolo Porto, Judith Kobler Waldis, and Christine Alewell

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Cited articles

Alewell, C., Meusburger, K., Juretzko, G., Mabit, L., and Ketterer, M. E.: Suitability of 239+240Pu and 137Cs as tracers for soil erosion assessment in mountain grasslands, Chemosphere, 103, 274–280, https://doi.org/10.1016/j.chemosphere.2013.12.016, 2014. 
Alewell, C., Birkholz, A., Meusburger, K., Schindler Wildhaber, Y., and Mabit, L.: Quantitative sediment source attribution with compound-specific isotope analysis in a C3 plant-dominated catchment (central Switzerland), Biogeosciences, 13, 1587–1596, https://doi.org/10.5194/bg-13-1587-2016, 2016. 
Alewell, C., Pitois, A., Meusburger, K., Ketterer, M., and Mabit, L.: Pu239+240 from “contaminant” to soil erosion tracer: Where do we stand?, Earth-Sci. Rev., 172, 107–123, https://doi.org/10.1016/j.earscirev.2017.07.009, 2017. 
Alewell, C., Ringeval, B., Ballabio, C., Robinson, D. A., Panagos, P., and Borrelli, P.: Global phosphorus shortage will be aggravated by soil erosion, Nat. Commun., 11, 4546, https://doi.org/10.1038/s41467-020-18326-7, 2020. 
Amundson, R., Berhe, A. A., Hopmans, J. W., Olson, C., Sztein, A. E., and Sparks, D. L.: Soil and human security in the 21st century, Science, 348, https://doi.org/10.1126/science.1261071, 2015. 
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Short summary
Quantifying soil redistribution rates is a global challenge. Radiogenic tracers such as plutonium, namely 239+240Pu, released to the atmosphere by atmospheric bomb testing in the 1960s are promising tools to quantify soil redistribution. Direct validation of 239+240Pu as soil redistribution is, however, still missing. Here, we used a unique sediment yield time series in southern Italy, reaching back to the initial fallout of 239+240Pu to verify 239+240Pu as a soil redistribution tracer.